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A Mechanoresponsive Phase‐Changing Electrolyte Enables Fabrication of High‐Output Solid‐State Photobioelectrochemical Devices from Pigment‐Protein Multilayers
Sai Kishore Ravi, David J. K. Swainsbury, Varun Kumar Singh, Yoke Keng Ngeow +2
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Abstract
, a fivefold improvement over the best previous comparable devices under standard illumination conditions. Photocurrent generation is enhanced by directional energy transfer through extended layers of light-harvesting complexes, mimicking the modular antenna/transducer architecture of natural photosystems, and by metastable radical pair formation when photovoltaic reaction centers are embedded throughout light-harvesting regions of the device.
Keywords
Materials sciencePhotocurrentElectrolyteOptoelectronicsQuasi-solidNanotechnologyPhotodiodeEnergy harvestingElectrodeDye-sensitized solar cellChemistry
Identifiers
- Journal
- Advanced Materials
- Year
- 2017